Tritium measurement using accelerator mass spectrometry and its application

Yuhua MA; Youshi ZENG; Wei LIU; Yan LI

doi:10.11889/j.1000-3436.2017.rrj.35.060101

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Tritium measurement using accelerator mass spectrometry and its application

REVIEW | 更新时间：2021-12-10

- Tritium measurement using accelerator mass spectrometry and its application
- Journal of Radiation Research and Radiation Processing Vol. 35, Issue 6, (2017)
- 作者机构：
  
  1.中国科学院上海应用物理研究所嘉定园区上海 201800
  2.中国科学院大学北京 100049
  3.上海科技大学上海 201200
- 作者简介：
- 基金信息：
  
  National Natural Science Foundation of China(11705265)
- DOI：10.11889/j.1000-3436.2017.rrj.35.060101
  CLC：
扫描看全文
Yuhua MA, Youshi ZENG, Wei LIU, et al. Tritium measurement using accelerator mass spectrometry and its application. [J]. Journal of Radiation Research and Radiation Processing 35(6):060101-7(2017)
DOI：

Yuhua MA, Youshi ZENG, Wei LIU, et al. Tritium measurement using accelerator mass spectrometry and its application. [J]. Journal of Radiation Research and Radiation Processing 35(6):060101-7(2017) DOI： 10.11889/j.1000-3436.2017.rrj.35.060101.

摘要

氚是环境中的主要放射性核素之一，对氚进行准确高效的监测是十分有必要的。目前常用的液体闪烁计数法所需的样品量较大，测量时间较长，不能对微量样品进行高精度测量。加速器质谱具有测量样品小、测量精度高和测量时间短的特点，能够更好地满足环境氚监测的需求，可以广泛应用于地球与环境科学、生物医学和辐射监测等方面。文中介绍了加速器质谱测氚的基本原理和发展历史、制样方法，对加速器质谱测氚的已有研究成果和主要应用进行了总结和展望。

Abstract

The demand for accurate and efficient tritium monitoring is growing rapidly as tritium has become one of the major radionuclides in the environment. Conventional methods based on liquid scintillation counting require long measurement time and tens of grams to kilograms of sample material, which limits the high-precision measurement of small-sized samples. To rapidly determine tritium concentrations from milligrams of sample material and therefore enable the accurate and efficient measurement of small-size environmental samples, accelerator mass spectrometry (AMS) is used for tritium determination. Hence, AMS tritium measurement is widely used in earth science, biomedicine, and radiation monitoring. In this paper, the basic principles and development history of tritium measurement by accelerator mass spectrometry are reviewed, and the preparation methods for tritium samples are introduced. The key researches and main applications of tritium measurement using accelerator mass spectrometry are also summarized, with a view on future developments in this area.

关键词

加速器质谱氚有机结合氚

Keywords

Accelerator mass spectrometryTritiumOrganically bond tritium

references

R L Hill , J R Johnson . Metabolism and dosimetry of tritium . Health Physics , 1993 . 65 (6 ):628 -647 . DOI:10.1097/00004032-199312000-00003http://doi.org/10.1097/00004032-199312000-00003 .

孟丹 , 王伟娟 , 文玮 , 等 . 植物中有机结合氚制样条件的实验研究 . 核技术 , 2016 . 39 (9 ):45 -50 . DOI:10.11889/j.0253-3219.2016.hjs.39.090302http://doi.org/10.11889/j.0253-3219.2016.hjs.39.090302 .

Dan MENG , Weijuan WANG , Wei WEN , 等 . Experimental study of organically bound tritium preparation condition in plant . Nuclear Techniques , 2016 . 39 (9 ):45 -50 . DOI:10.11889/j.0253-3219.2016.hjs.39.090302http://doi.org/10.11889/j.0253-3219.2016.hjs.39.090302 .

R A Müller . Radioisotope dating with a cyclotron . Science , 1977 . 196 (4289 ):489 -494 . DOI:10.1126/science.196.4289.489http://doi.org/10.1126/science.196.4289.489 .

S E King , G W Phillips , R A August , 等 . Detection of tritium using accelerator mass spectrometry . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 1987 . 29 (1 ):14 -17 . DOI:10.1016/0168-583X(87)90194-7http://doi.org/10.1016/0168-583X(87)90194-7 .

B G Glagola , G W Phillips , K W Marlow , 等 . Low level tritium detection using accelerator mass spectrometry . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 1984 . 5 (2 ):221 -225 . DOI:10.1016/0168-583X(84)90514-7http://doi.org/10.1016/0168-583X(84)90514-7 .

S Jiang , A Yu , Y Cui , 等 . Determination of tritium using a small Van de Graaff accelerator . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 1984 . 5 (2 ):226 -229 . DOI:10.1016/0168-583X(84)90515-9http://doi.org/10.1016/0168-583X(84)90515-9 .

周善铸 , 潘浩昌 , 林俊英 , 等 . 应用回旋加速器测量水中微量氚 . 核技术 , 1984 . 7 (5 ):30 -32+73 . http://kns.cnki.net/KCMS/detail/detail.aspx?filename=hjsu198405008&dbname=CJFD&dbcode=CJFQhttp://kns.cnki.net/KCMS/detail/detail.aspx?filename=hjsu198405008&dbname=CJFD&dbcode=CJFQ, .

Shanzhu ZHOU , Haochang PAN , Junying LIN , 等 . Measurement of 3H content in water sample with a cyclotron . Nuclear Techniques , 1984 . 7 (5 ):30 -32+73 . http://kns.cnki.net/KCMS/detail/detail.aspx?filename=hjsu198405008&dbname=CJFD&dbcode=CJFQhttp://kns.cnki.net/KCMS/detail/detail.aspx?filename=hjsu198405008&dbname=CJFD&dbcode=CJFQ, .

R Middleton , J Klein , D Fink . Tritium measurements with a tandem accelerator . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 1990 . 47 (4 ):409 -414 . DOI:10.1016/0168-583X(90)90619-6http://doi.org/10.1016/0168-583X(90)90619-6 .

M L Chiarappa-Zucca , K H Dingley , M L Roberts , 等 . Sample preparation for quantitation of tritium by accelerator mass spectrometry . Analytical Chemistry , 2002 . 74 (24 ):6285 -6290 . DOI:10.1021/ac020295uhttp://doi.org/10.1021/ac020295u .

Ognibene T J, Vogel J S. Highly sensitive 14C and 3H quantification of biochemical samples using accelerator mass spectrometry[R]. Lawrence Livermore National Laboratory (LLNL), Livermore, CA, 2003.https://www.researchgate.net/publication/241959660_Highly_Sensitive_14C_and_3H_Quantification_of_Biochemical_Samples_Using_Accelerator_Mass_Spectrometry

A H Love , J R Hunt , M L Roberts , 等 . Use of tritium accelerator mass spectrometry for tree ring analysis . Environmental Science & Technology , 2002 . 36 (13 ):2848 -2852 . DOI:10.1021/es015837ohttp://doi.org/10.1021/es015837o .

A H Love , J R Hunt , J P Knezovich . Reconstructing tritium exposure using tree rings at Lawrence Berkeley National Laboratory, California . Environmental Science & Technology , 2003 . 37 (19 ):4330 -4335 . DOI:10.1021/es034278dhttp://doi.org/10.1021/es034278d .

Purser K H. Miniature AMS detector for ultrasensitive detection of individual carbon-14 and tritium atoms:U.S. Patent 5, 661, 299[P]. 1997-8-26.http://www.google.com/patents/US5661299?hl=zh-CN

J Heinemeier , J Olsen , M Klein , 等 . The new extended HVE 1MV multi-element AMS system for low background installed at the Aarhus AMS Dating Centre . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 2015 . 361 143 -148 . DOI:10.1016/j.nimb.2015.05.039http://doi.org/10.1016/j.nimb.2015.05.039 .

王华 , 殷建军 , 杨会 , 等 . 聚合膜电解浓集法测量低水平氚环境水样的氚比活度 . 岩矿测试 , 2011 . 30 (6 ):745 -750 . DOI:10.15898/j.cnki.11-2131/td.2011.06.016http://doi.org/10.15898/j.cnki.11-2131/td.2011.06.016 .

Hua WANG , Jianjun YIN , Hui YANG , 等 . Application of the solid polymer electrolysis enrichment method for low level tritium in environmental water and the calculation of tritium specific activity . Rock and Mineral Analysis , 2011 . 30 (6 ):745 -750 . DOI:10.15898/j.cnki.11-2131/td.2011.06.016http://doi.org/10.15898/j.cnki.11-2131/td.2011.06.016 .

杨海兰 . 液体闪烁计数与低水平环境氚的监测 . 辐射防护通讯 , 2012 . 32 (1 ):1 -7, 27 . http://kns.cnki.net/KCMS/detail/detail.aspx?filename=defe201201002&dbname=CJFD&dbcode=CJFQhttp://kns.cnki.net/KCMS/detail/detail.aspx?filename=defe201201002&dbname=CJFD&dbcode=CJFQ, .

Hailan YANG . Liquid scintillation counting and tritium monitoring in the environment . Radiation Protection Bulletin , 2012 . 32 (1 ):1 -7, 27 . http://kns.cnki.net/KCMS/detail/detail.aspx?filename=defe201201002&dbname=CJFD&dbcode=CJFQhttp://kns.cnki.net/KCMS/detail/detail.aspx?filename=defe201201002&dbname=CJFD&dbcode=CJFQ, .

G Etiope , Lollar B Sherwood . Abiotic methane on earth . Reviews of Geophysics , 2013 . 51 (2 ):276 -299 . DOI:10.1002/rog.20011http://doi.org/10.1002/rog.20011 .

M Schoell . Multiple origins of methane in the Earth . Chemical Geology , 1988 . 71 (1-3 ):1 -10 . DOI:10.1016/0009-2541(88)90101-5http://doi.org/10.1016/0009-2541(88)90101-5 .

M J Whiticar . Carbon and hydrogen isotope systematics of bacterial formation and oxidation of methane . Chemical Geology , 1999 . 161 (1 ):291 -314 . DOI:10.1016/S0009-2541(99)00092-3http://doi.org/10.1016/S0009-2541(99)00092-3 .

K Brown , K H Dingley , K W Turteltaub . Accelerator mass spectrometry for biomedical research . Methods in Enzymology , 2005 . 402 423 -443 . DOI:10.1016/S0076-6879(05)02014-8http://doi.org/10.1016/S0076-6879(05)02014-8 .

K H Dingley , M L Roberts , C A Velsko , 等 . Attomole detection of 3H in biological samples using accelerator mass spectrometry:application in low-dose, dual-isotope tracer studies in conjunction with 14C accelerator mass spectrometry . Chemical Research in Toxicology , 1998 . 11 (10 ):1217 -1222 . DOI:10.1021/tx9801458http://doi.org/10.1021/tx9801458 .

K H Dingley , E A Ubick , M L Chiarappa-Zucca , 等 . Effect of dietary constituents with chemopreventive potential on adduct formation of a low dose of the heterocyclic amines PhIP and IQ and phase Ⅱ hepatic enzymes . Nutrition Cancer , 2003 . 46 (2 ):212 -221 . DOI:10.1207/S15327914NC4602_15http://doi.org/10.1207/S15327914NC4602_15 .

Y Yamada , K Yasuike , K Komura . Temporal variation of tritium concentration in tree-ring cellulose over the past 50 years . Journal of Radioanalytical and Nuclear Chemistry , 2004 . 262 (3 ):679 -683 . DOI:10.1007/s10967-004-0492-9http://doi.org/10.1007/s10967-004-0492-9 .

M Friedrich , G Sun , R Grötzschel , 等 . Tritium depth profiling in carbon by accelerator mass spectrometry . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 1997 . 123 (1-4 ):410 -413 . DOI:10.1016/S0168-583X(96)00404-1http://doi.org/10.1016/S0168-583X(96)00404-1 .

M Friedrich , W Pilz , G Sun , 等 . Tritium depth profiling in carbon by accelerator mass spectrometry . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 2000 . 161 216 -220 . DOI:10.1016/S0168-583X(99)00678-3http://doi.org/10.1016/S0168-583X(99)00678-3 .

C Stan-Sion , N Bekris , G Kizane , 等 . Tritium retention measurements by accelerator mass spectrometry and full combustion of W-coated and uncoated CFC tiles from the JET divertor . Nuclear Fusion , 2016 . 56 (4 ):046015 DOI:10.1088/0029-5515/56/4/046015http://doi.org/10.1088/0029-5515/56/4/046015 .

W Pilz , M Friedrich , K H Heinig , 等 . AMS depth profiling of humidity in silica . Nuclear Instruments and Methods in Physics Research Section B:Beam Interactions with Materials and Atoms , 2004 . 219 459 -462 . DOI:10.1016/j.nimb.2004.01.102http://doi.org/10.1016/j.nimb.2004.01.102 .

Roberts M L, Davis J C. Small system for tritium accelerator mass spectrometry:U.S. Patent 5, 189, 302[P]. 1993-2-23.

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